Menu
Publications
2025
2024
2023
2022
2021
2020
2019
2018
2017
2016
2015
2014
2013
2012
2011
2010
2009
2008
2007
2006
2005
2004
2003
2002
2001
Editor-in-Chief

Nikiforov
Vladimir O.
D.Sc., Prof.
Partners
doi: 10.17586/2226-1494-2022-22-4-635-642
Investigation of congruent lithium niobate crystal dispersion properties in the terahertz frequency range
Read the full article

Article in Russian
For citation:
Abstract
For citation:
Shumigai V.S., Oparin E.N., Nabilkova A.O., Melnik M.V., Tcypkin A.N., Kozlov S.A. Investigation of congruent lithium niobate crystal dispersion properties in the terahertz frequency range. Scientific and Technical Journal of Information Technologies, Mechanics and Optics, 2022, vol. 22, no. 4, pp. 635–642 (in Russian). doi: 10.17586/2226-1494-2022-22-4-635-642
Abstract
Dispersion curves of the refraction index of a congruent lithium niobate (cLN) crystal cut perpendicular to the x and z axes in the terahertz frequency range are considered. In the study, the method of terahertz time domain spectroscopy with time resolution is used passed through an initially isotropic detecting crystal which becomes birefringent when exposed to a terahertz field. The magnitude of the induced birefringence is proportional to the amplitude of the terahertz field. Using Fourier analysis of a terahertz pulse passing through a cLN crystal and a reference pulse that does not interact with the object, the frequency dependences of the refractive index and the absorption coefficient of the object under study are constructed. Dispersion curves are presented for the real part of the refractive index of a cLN crystal cut along the planes (100) and (001), in the frequency range 0.25–1.25 THz. Simulation of the propagation of a one-and-a-half-cycle pulse in media with dispersion is performed based on the data of scientific papers by other authors. As a result, the temporal forms of the output signals are found. Conclusion about the inaccuracy of the dispersion curves from the selected works is made. The parameters has been identified whose optimization made it possible to eliminate inaccuracies in the display of the dispersion dependence for the high-frequency region of the terahertz spectrum were identified. The results obtained are very important for the design of devices based on nonlinear optical effects. These data will be useful for the generation of difference frequencies, optical rectification and generation of terahertz radiation as well as for areas where accurate data on the terahertz dispersion properties of nonlinear crystals, including cLN, are required.
Keywords: terahertz radiation, dispersion, congruent crystal, lithium niobate, terahertz time-domain spectroscopy, refractive index
Acknowledgements. This work was supported by the Ministry of Science and Education of the Russian Federation (Passport No. 2019-0903).
References
Acknowledgements. This work was supported by the Ministry of Science and Education of the Russian Federation (Passport No. 2019-0903).
References
-
Glagolewa-Arkadiewa A. Short electromagnetic waves of wave-length up to 82 microns. Nature, 1924, vol. 113, no. 2844, pp. 640–640. https://doi.org/10.1038/113640a0
-
Evenson K.M., Wells J.S., Matarrese L.M. Absolute Frequency Measurements of The CO2 CW Laser at 28 THz (10.6μm). Applied Physics Letters,1970, vol. 16, no. 6, pp. 251–253. https://doi.org/10.1063/1.1653183
-
Hangyo M., Tani M., Nagashima T. Terahertz time-domain spectroscopy of solids: A review. International Journal of Infrared and Millimeter Waves, 2005, vol. 26,no. 12, pp. 1661–1690. https://doi.org/10.1007/s10762-005-0288-1
-
Liu M.K., Hwang H.Y., Tao H., Strikwerda A.C., Fan K.B., Keiser G.R., Sternbach A.J., West K.G., Kittiwatanakul S., Lu J.W., Wolf S.A., Omenetto F.G., Zhang X., Nelson K.A., Averitt R.D. Terahertz-field-induced insulator-to-metal transition in vanadium dioxide metamaterial. Nature, 2012, vol. 487, no. 7407, pp. 345–348. https://doi.org/10.1038/nature11231
-
Tcypkin A.N., Melnik M.V., Zhukova M.O., Vorontsova I.O., Putilin S.E., Kozlov S.A., Zhang X.-C. High Kerr nonlinearity of water in THz spectral range. Optics express, 2019, vol. 27, no. 8, pp. 10419–10425. https://doi.org/10.1364/OE.27.010419
-
Tcypkin A., Zhukova M., Vorontsova I., Kulya M., Putilin S., Kozlov S., Choudhary S., Boyd R.W. Giant third-order nonlinear response of liquids at terahertz frequencies. Physical Review Applied, 2021, vol. 15, no. 5, pp. 054009. https://doi.org/10.1103/PhysRevApplied.15.054009
-
Kawase K., Sato M., Taniuchi T., Ito H. Coherent tunable THz‐wave generation from LiNbO3 with monolithic grating coupler. Applied Physics Letters, 1996, vol. 68, no. 18, pp. 2483–2485. https://doi.org/10.1063/1.115828
-
Bodrov S.B., Ilyakov I.E., Shishkin B.V., Stepanov A.N. Efficient terahertz generation by optical rectification in Si-LiNbO3-air-metal sandwich structure with variable air gap. Applied Physics Letters, 2012, vol. 100, no. 20, pp. 201114. https://doi.org/10.1063/1.4719674
-
Nagashima K., Kosuge A. Design of rectangular transmission gratings fabricated in LiNbO3 for high-power terahertz-wave generation. Japanese Journal of Applied Physics, 2010, vol. 49, no. 12R, pp. 122504. https://doi.org/10.1143/JJAP.49.122504
-
Zhukova M., Melnik M., Vorontsova I., Tcypkin A., Kozlov S. Estimations of low-inertia cubic nonlinearity featured by electro-optical crystals in the thz range. Photonics, 2020, vol. 7, no. 4, pp. 98. https://doi.org/10.3390/photonics7040098
-
Neu J., Schmuttenmaer C.A. Tutorial: An introduction to terahertz time domain spectroscopy (THz-TDS). Journal of Applied Physics, 2018, vol. 124, no. 23, pp. 231101. https://doi.org/10.1063/1.5047659
-
Peretti R., Mitryukovskiy S., Froberger K., Mebarki M.A., Eliet S., Vanwolleghem M., Lampin J.-F. THz-TDS time-trace analysis for the extraction of material and metamaterial parameters. IEEE Transactions on Terahertz Science and Technology, 2018, vol. 9, no. 2, pp. 136–149. https://doi.org/10.1109/TTHZ.2018.2889227
-
Nahata A., Weling A.S., Heinz T.F. A wideband coherent terahertz spectroscopy system using optical rectification and electro‐optic sampling. Applied Physics Letters, 1996, vol. 69, no. 16, pp. 2321–2323. https://doi.org/10.1063/1.117511
-
Pálfalvi L., Hebling J., Kuhl J., Ṕter Á., Polgár K. Temperature dependence of the absorption and refraction of Mg-doped congruent and stoichiometric LiNbO3 in the THz range. Journal of Applied Physics, 2005, vol. 97, no. 12, pp. 123505. https://doi.org/10.1063/1.1929859
-
Wang T.D., Lin S.T., Lin Y.Y., Chiang A.C., Huang Y.C. Forward and backward terahertz-wave difference-frequency generations from periodically poled lithium niobate. Optics Express, 2008, vol. 16, no. 9, pp. 6471–6478. https://doi.org/10.1364/OE.16.006471
-
Drozdov A., Kozlov S. Phase self-modulation of single-cycle optical waves. Scientific and Technical Journal of Information Technologies, Mechanics and Optics, 2011, no. 2(72), pp. 99–105. (in Russian)
-
Grachev Y.V., Osipova M.O., Kuz'mina A.V., Bespalov V.G. Determining the working band of frequencies of a pulsed terahertz spectrometer. Journal of Optical Technology, 2014, vol. 81, no. 8, pp. 468–471. https://doi.org/10.1364/JOT.81.000468
-
Li D., Ma G., Ge J., Hu S., Dai N. Terahertz pulse shaping via birefringence in lithium niobate crystal. Applied Physics B, 2009, vol. 94, no. 4, pp. 623–628. https://doi.org/10.1007/s00340-008-3334-6
-
Unferdorben M., Szaller Z., Hajdara I., Hebling J., Pálfalvi L. Measurement of refractive index and absorption coefficient of congruent and stoichiometric lithium niobate in the terahertz range. Journal of Infrared, Millimeter, and Terahertz Waves, 2015, vol. 36, no. 12, pp. 1203–1209. https://doi.org/10.1007/s10762-015-0165-5
-
Mao Z.-L., Hou B.-H., Wang L., Sun Y.-M., Hao W. The study of the terahertz spectral of LiNbO3 crystal. Proc. of the Joint 31st International Conference on Infrared Millimeter Waves and 14th International Conference on Teraherz Electronics, 2006, pp. 465–465. https://doi.org/10.1109/ICIMW.2006.368673
-
Samartcev V., Kozlov S. Basics of Femtosecond Optics. Moscow, Fizmatlit Publ., 2009, 292 с. (in Russian)